Abstract:
The nonlinear interaction of $250$-fs laser pulses at a wavelength of $1030$ nm with polymethyl methacrylate is investigated using an optimized $z$-scan technique. It is shown that the mechanism of pulse attenuation for peak intensities below $0.65$ TW/cm$^2$ can be described as four-photon absorption with the coefficient $\beta_4 = (35\pm5)$ cm$^5$/TW$^3$. The nonlinear refractive index ${n_2} = (7.6\pm0.4)\times10^{-4}$ cm$^2$/TW and the critical power for the onset of self-focusing $P_{\text{cr}}= (1.42\pm0.08)$ MW are determined and these results are used to demonstrate the correspondence between the calculated shift of the nonlinear focal point and the location of the laser-modified regions.